bibtype J - Journal Article
ARLID 0579532
utime 20240402214919.0
mtime 20231214235959.9
SCOPUS 85180599822
WOS 001168847100001
DOI 10.5194/acp-23-15235-2023
title (primary) (eng) Decreasing trends of ammonia emissions over Europe seen from remote sensing and inverse modelling
specification
page_count 18 s.
media_type P
serial
ARLID cav_un_epca*0257783
ISSN 1680-7316
title Atmospheric Chemistry and Physics
volume_id 23
volume 24 (2023)
page_num 15235-15252
publisher
name Copernicus
keyword ammonia emissions
keyword inverse modelling
keyword remote sensing
author (primary)
ARLID cav_un_auth*0267768
name1 Tichý
name2 Ondřej
institution UTIA-B
full_dept (cz) Adaptivní systémy
full_dept (eng) Department of Adaptive Systems
department (cz) AS
department (eng) AS
full_dept Department of Adaptive Systems
fullinstit Ústav teorie informace a automatizace AV ČR, v. v. i.
author
ARLID cav_un_auth*0419235
name1 Eckhardt
name2 S.
country NO
author
ARLID cav_un_auth*0450270
name1 Balkanski
name2 Y.
country FR
author
ARLID cav_un_auth*0450271
name1 Hauglustaine
name2 D.
country FR
author
ARLID cav_un_auth*0363740
name1 Evangeliou
name2 N.
country NO
source
url http://library.utia.cas.cz/separaty/2023/AS/tichy-0579532.pdf
source
url https://acp.copernicus.org/articles/23/15235/2023/
cas_special
project
project_id GA20-27939S
agency GA ČR
ARLID cav_un_auth*0391986
abstract (eng) Ammonia (NH3), a significant precursor of particulate matter, affects not only biodiversity, ecosystems, and soil acidification but also climate and human health. In addition, its concentrations are constantly rising due to increasing feeding needs and the large use of fertilization and animal farming. Despite the significance of ammonia, its emissions are associated with large uncertainties, while its atmospheric abundance is difficult to measure. Nowadays, satellite products can effectively measure ammonia with low uncertainty and a global coverage. Here, we use satellite observations of column ammonia in combination with an inversion algorithm to derive ammonia emissions with a high resolution over Europe for the period 2013–2020. Ammonia emissions peak in northern Europe due to agricultural application and livestock management, in western Europe (industrial activity), and over Spain (pig farming). Emissions have decreased by −26 % since 2013 (from 5431 Gg in 2013 to 3994 Gg in 2020), showing that the abatement strategies adopted by the European Union have been very efficient. The slight increase (+4.4 %) in 2015 is also reproduced here and is attributed to some European countries exceeding annual emission targets. Ammonia emissions are low in winter (286 Gg) and peak in summer (563 Gg) and are dominated by the temperature-dependent volatilization of ammonia from the soil. The largest emission decreases were observed in central and eastern Europe (−38 %) and in western Europe (−37 %), while smaller decreases were recorded in northern (−17 %) and southern Europe (−7.6 %). When complemented with ground observations, modelled concentrations using the posterior emissions showed improved statistics, also following the observed seasonal trends. The posterior emissions presented here also agree well with respective estimates reported in the literature and inferred from bottom-up and top-down methodologies. These results indicate that satellite measurements combined with inverse algorithms constitute a robust tool for emission estimates and can infer the evolution of ammonia emissions over large timescales.
result_subspec WOS
RIV BB
FORD0 10000
FORD1 10500
FORD2 10509
reportyear 2024
num_of_auth 5
inst_support RVO:67985556
permalink https://hdl.handle.net/11104/0348911
confidential S
mrcbC91 A
mrcbT16-e ENVIRONMENTALSCIENCES|METEOROLOGYATMOSPHERICSCIENCES
mrcbT16-j 1.59
mrcbT16-s 2.463
mrcbT16-D Q1
mrcbT16-E Q1*
arlyear 2023
mrcbU14 85180599822 SCOPUS
mrcbU24 PUBMED
mrcbU34 001168847100001 WOS
mrcbU63 cav_un_epca*0257783 Atmospheric Chemistry and Physics Roč. 23 č. 24 2023 15235 15252 1680-7316 1680-7324 Copernicus